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QIN, SJ; YOU, WM; SU, ZB; QIN, SJ , ACAD SINICA,INST THEORET PHYS,POB 2735,BEIJING 100080,PEOPLES R CHINA.
2ND-HARMONIC GENERATION FROM THE QUADRUPOLE RESPONSE IN C-60 FILMS
Source PublicationPHYSICAL REVIEW B
KeywordMolecular-orientation Optical-absorption C-60 Carbon Excitations Model
AbstractBy applying the numerically computed energy levels and wave functions of the pi electrons of the C60 molecule following the Su-Schrieffer-Heeger model, we calculated the second-order quadrupole nonlinear susceptibility x(zzzz)Q for the C60 medium and the calculated value is 1.7 X 10(-20) m2/V for the fundamental wave lambda = 1.064 mum. For the fundamental wave lambda = 1.064 mum, the second-order susceptibility chi(zzz)(2) caused by the second-order nonlinear quadrupole polarization has the magnitude 1.1 X 10(-13) m/V (i.e., 2.5 X 10(-9) esu). This result is in excellent agreement with the recent experimental measurements. In addition, we also calculated the quadrupole-induced reflection and transmission second-order harmonic generation by further considering the effect of finite film thickness.
1993
ISSN1098-0121
Volume48Issue:23Pages:17562-17568
Subject AreaPhysics
Indexed BySCI
Document Type期刊论文
Identifierhttp://ir.itp.ac.cn/handle/311006/11976
Collection理论物理所科研产出_SCI论文
Corresponding AuthorQIN, SJ , ACAD SINICA,INST THEORET PHYS,POB 2735,BEIJING 100080,PEOPLES R CHINA.
Recommended Citation
GB/T 7714
QIN, SJ,YOU, WM,SU, ZB,et al. 2ND-HARMONIC GENERATION FROM THE QUADRUPOLE RESPONSE IN C-60 FILMS[J]. PHYSICAL REVIEW B,1993,48(23):17562-17568.
APA QIN, SJ,YOU, WM,SU, ZB,&QIN, SJ , ACAD SINICA,INST THEORET PHYS,POB 2735,BEIJING 100080,PEOPLES R CHINA..(1993).2ND-HARMONIC GENERATION FROM THE QUADRUPOLE RESPONSE IN C-60 FILMS.PHYSICAL REVIEW B,48(23),17562-17568.
MLA QIN, SJ,et al."2ND-HARMONIC GENERATION FROM THE QUADRUPOLE RESPONSE IN C-60 FILMS".PHYSICAL REVIEW B 48.23(1993):17562-17568.
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