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题名: 2ND-HARMONIC GENERATION FROM THE QUADRUPOLE RESPONSE IN C-60 FILMS
作者: QIN, SJ ;  YOU, WM ;  SU, ZB
刊名: PHYSICAL REVIEW B
出版日期: 1993
卷号: 48, 期号:23, 页码:17562-17568
关键词: MOLECULAR-ORIENTATION ;  OPTICAL-ABSORPTION ;  C-60 ;  CARBON ;  EXCITATIONS ;  MODEL
学科分类: Physics
通讯作者: QIN, SJ , ACAD SINICA,INST THEORET PHYS,POB 2735,BEIJING 100080,PEOPLES R CHINA.
英文摘要: By applying the numerically computed energy levels and wave functions of the pi electrons of the C60 molecule following the Su-Schrieffer-Heeger model, we calculated the second-order quadrupole nonlinear susceptibility x(zzzz)Q for the C60 medium and the calculated value is 1.7 X 10(-20) m2/V for the fundamental wave lambda = 1.064 mum. For the fundamental wave lambda = 1.064 mum, the second-order susceptibility chi(zzz)(2) caused by the second-order nonlinear quadrupole polarization has the magnitude 1.1 X 10(-13) m/V (i.e., 2.5 X 10(-9) esu). This result is in excellent agreement with the recent experimental measurements. In addition, we also calculated the quadrupole-induced reflection and transmission second-order harmonic generation by further considering the effect of finite film thickness.
收录类别: SCI
原文出处: 查看原文
内容类型: 期刊论文
URI标识: http://ir.itp.ac.cn/handle/311006/11976
Appears in Collections:理论物理所1978-2010年知识产出_期刊论文

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Recommended Citation:
QIN, SJ,YOU, WM,SU, ZB. 2ND-HARMONIC GENERATION FROM THE QUADRUPOLE RESPONSE IN C-60 FILMS[J]. PHYSICAL REVIEW B,1993,48(23):17562-17568.
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