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2ND-HARMONIC GENERATION FROM THE QUADRUPOLE RESPONSE IN C-60 FILMS
QIN, SJ; YOU, WM; SU, ZB; QIN, SJ , ACAD SINICA,INST THEORET PHYS,POB 2735,BEIJING 100080,PEOPLES R CHINA.
1993
发表期刊PHYSICAL REVIEW B
ISSN1098-0121
卷号48期号:23页码:17562-17568
摘要By applying the numerically computed energy levels and wave functions of the pi electrons of the C60 molecule following the Su-Schrieffer-Heeger model, we calculated the second-order quadrupole nonlinear susceptibility x(zzzz)Q for the C60 medium and the calculated value is 1.7 X 10(-20) m2/V for the fundamental wave lambda = 1.064 mum. For the fundamental wave lambda = 1.064 mum, the second-order susceptibility chi(zzz)(2) caused by the second-order nonlinear quadrupole polarization has the magnitude 1.1 X 10(-13) m/V (i.e., 2.5 X 10(-9) esu). This result is in excellent agreement with the recent experimental measurements. In addition, we also calculated the quadrupole-induced reflection and transmission second-order harmonic generation by further considering the effect of finite film thickness.
关键词Molecular-orientation Optical-absorption C-60 Carbon Excitations Model
学科领域Physics
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收录类别SCI
文献类型期刊论文
条目标识符http://ir.itp.ac.cn/handle/311006/11976
专题理论物理所SCI论文
通讯作者QIN, SJ , ACAD SINICA,INST THEORET PHYS,POB 2735,BEIJING 100080,PEOPLES R CHINA.
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QIN, SJ,YOU, WM,SU, ZB,et al. 2ND-HARMONIC GENERATION FROM THE QUADRUPOLE RESPONSE IN C-60 FILMS[J]. PHYSICAL REVIEW B,1993,48(23):17562-17568.
APA QIN, SJ,YOU, WM,SU, ZB,&QIN, SJ , ACAD SINICA,INST THEORET PHYS,POB 2735,BEIJING 100080,PEOPLES R CHINA..(1993).2ND-HARMONIC GENERATION FROM THE QUADRUPOLE RESPONSE IN C-60 FILMS.PHYSICAL REVIEW B,48(23),17562-17568.
MLA QIN, SJ,et al."2ND-HARMONIC GENERATION FROM THE QUADRUPOLE RESPONSE IN C-60 FILMS".PHYSICAL REVIEW B 48.23(1993):17562-17568.
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