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Wang, WZ; Wang, CL; Bishop, AR; Yu, L; Su, ZB; Wang, WZ , LOS ALAMOS NATL LAB,DIV THEORET,LOS ALAMOS,NM 87545, USA.
Dynamic Jahn-Teller effect in fullerene C-60 and related observable effects
发表期刊SYNTHETIC METALS
关键词Electron-vibron Interactions Charged Fullerenes Berry Phases C60 Triplet Absorption Molecules Spectra Anion State
摘要Based on the Bogoliubov-de Gennes formalism, the linear multi-mode T-1u circle times 8h(g) static Jahn-Teller problem is aanalyzed for the charged C-60(-), C-60(2-), the lowest triplet and singlet self-trapped exciton (STE) of C-60. The dynamic Jahn-Teller effect due to quantum tunneling between the six degenerate D-5d configurations is studied within a perturbation approach. The tunneling induced level splittings are determined to be T-2(1u) circle plus T-2(3u), (1)A(g) circle plus H-1(g), T-3(3g) circle plus T-3(1g) and T-1(3g) circle plus T-1(1g) for C-60(1-), C-60(2-), triplet and singlet STE's of neutral C-60, respectively. The observable consequences of the dynamic Jahn-Teller effect are considered. Some of the Jahn-Teller active (as well as Raman-active) modes are predicted to be observable as multi-phonon overtones in the infrared absorption. In the photo-induced multi-phonon resonant Raman scattering the tunnel splitting itself should show up in the Raman spectrum, and the depolarization ratio is sensitive to the exciting frequency.
1997
ISSN0379-6779
卷号86期号:40911页码:2365-2368
学科领域Physics
收录类别SCI
引用统计
被引频次:4[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.itp.ac.cn/handle/311006/12510
专题理论物理所科研产出_SCI论文
通讯作者Wang, WZ , LOS ALAMOS NATL LAB,DIV THEORET,LOS ALAMOS,NM 87545, USA.
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Wang, WZ,Wang, CL,Bishop, AR,et al. Dynamic Jahn-Teller effect in fullerene C-60 and related observable effects[J]. SYNTHETIC METALS,1997,86(40911):2365-2368.
APA Wang, WZ,Wang, CL,Bishop, AR,Yu, L,Su, ZB,&Wang, WZ , LOS ALAMOS NATL LAB,DIV THEORET,LOS ALAMOS,NM 87545, USA..(1997).Dynamic Jahn-Teller effect in fullerene C-60 and related observable effects.SYNTHETIC METALS,86(40911),2365-2368.
MLA Wang, WZ,et al."Dynamic Jahn-Teller effect in fullerene C-60 and related observable effects".SYNTHETIC METALS 86.40911(1997):2365-2368.
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