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Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression
Iwamoto, M; Wu, CX; Zhong-Can, OY; Iwamoto, M , Tokyo Inst Technol, Dept Phys Elect, Meguro Ku, 2-12-1 Ookayama, Tokyo 1528552, Japan.
2000
发表期刊CHEMICAL PHYSICS LETTERS
ISSN0009-2614
卷号325期号:41035页码:545-551
摘要The complete expression for the macroscopic second-order susceptibility (SOS) tensor chi((2)) for a monolayer with C-infinity symmetry at the air-liquid interface is derived as functions of the molecular SOS tensor alpha((2)) and the orientational order parameters. The chiral (non-chiral) terms of chi((2)) distinguished by their association with even (odd) order parameters, by which a second-harmonic generation (SHG) circular-dichroism effect can be better understood. An SHG experiment of a 4-cyano-4'-5-alkyl-biphenyl monolayer on an air-water interface by monolayer compression is also discussed. (C) 2000 Elsevier Science B.V. All rights reserved.
部门归属Tokyo Inst Technol, Dept Phys Elect, Meguro Ku, Tokyo 1528552, Japan; Acad Sinica, Inst Theoret Phys, Beijing 100080, Peoples R China; Tsing Hua Univ, Ctr Adv Study, Beijing 100084, Peoples R China
关键词Circular-dichroism Spectroscopy Optical 2nd-harmonic Generation 2nd Harmonic-generation Molecular-orientation Rotational Averages Surface Films
学科领域Physics
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收录类别SCI
WOS记录号WOS:000088612600011
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被引频次:33[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.itp.ac.cn/handle/311006/12921
专题理论物理所1978-2010年知识产出
通讯作者Iwamoto, M , Tokyo Inst Technol, Dept Phys Elect, Meguro Ku, 2-12-1 Ookayama, Tokyo 1528552, Japan.
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Iwamoto, M,Wu, CX,Zhong-Can, OY,et al. Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression[J]. CHEMICAL PHYSICS LETTERS,2000,325(41035):545-551.
APA Iwamoto, M,Wu, CX,Zhong-Can, OY,&Iwamoto, M , Tokyo Inst Technol, Dept Phys Elect, Meguro Ku, 2-12-1 Ookayama, Tokyo 1528552, Japan..(2000).Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression.CHEMICAL PHYSICS LETTERS,325(41035),545-551.
MLA Iwamoto, M,et al."Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression".CHEMICAL PHYSICS LETTERS 325.41035(2000):545-551.
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