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Iwamoto, M; Wu, CX; Zhong-Can, OY; Iwamoto, M , Tokyo Inst Technol, Dept Phys Elect, Meguro Ku, 2-12-1 Ookayama, Tokyo 1528552, Japan.
Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression
Source PublicationCHEMICAL PHYSICS LETTERS
KeywordCircular-dichroism Spectroscopy Optical 2nd-harmonic Generation 2nd Harmonic-generation Molecular-orientation Rotational Averages Surface Films
AbstractThe complete expression for the macroscopic second-order susceptibility (SOS) tensor chi((2)) for a monolayer with C-infinity symmetry at the air-liquid interface is derived as functions of the molecular SOS tensor alpha((2)) and the orientational order parameters. The chiral (non-chiral) terms of chi((2)) distinguished by their association with even (odd) order parameters, by which a second-harmonic generation (SHG) circular-dichroism effect can be better understood. An SHG experiment of a 4-cyano-4'-5-alkyl-biphenyl monolayer on an air-water interface by monolayer compression is also discussed. (C) 2000 Elsevier Science B.V. All rights reserved.
2000
ISSN0009-2614
Volume325Issue:41035Pages:545-551
Subject AreaPhysics
Indexed BySCI
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Cited Times:33[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.itp.ac.cn/handle/311006/12921
Collection理论物理所科研产出_SCI论文
Corresponding AuthorIwamoto, M , Tokyo Inst Technol, Dept Phys Elect, Meguro Ku, 2-12-1 Ookayama, Tokyo 1528552, Japan.
Recommended Citation
GB/T 7714
Iwamoto, M,Wu, CX,Zhong-Can, OY,et al. Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression[J]. CHEMICAL PHYSICS LETTERS,2000,325(41035):545-551.
APA Iwamoto, M,Wu, CX,Zhong-Can, OY,&Iwamoto, M , Tokyo Inst Technol, Dept Phys Elect, Meguro Ku, 2-12-1 Ookayama, Tokyo 1528552, Japan..(2000).Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression.CHEMICAL PHYSICS LETTERS,325(41035),545-551.
MLA Iwamoto, M,et al."Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression".CHEMICAL PHYSICS LETTERS 325.41035(2000):545-551.
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