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| Iwamoto, M; Wu, CX; Zhong-Can, OY; Iwamoto, M , Tokyo Inst Technol, Dept Phys Elect, Meguro Ku, 2-12-1 Ookayama, Tokyo 1528552, Japan. | |
| Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression | |
| Source Publication | CHEMICAL PHYSICS LETTERS
 |
| Keyword | Circular-dichroism Spectroscopy Optical 2nd-harmonic Generation 2nd Harmonic-generation Molecular-orientation Rotational Averages Surface Films |
| Abstract | The complete expression for the macroscopic second-order susceptibility (SOS) tensor chi((2)) for a monolayer with C-infinity symmetry at the air-liquid interface is derived as functions of the molecular SOS tensor alpha((2)) and the orientational order parameters. The chiral (non-chiral) terms of chi((2)) distinguished by their association with even (odd) order parameters, by which a second-harmonic generation (SHG) circular-dichroism effect can be better understood. An SHG experiment of a 4-cyano-4'-5-alkyl-biphenyl monolayer on an air-water interface by monolayer compression is also discussed. (C) 2000 Elsevier Science B.V. All rights reserved. |
| 2000 | |
| ISSN | 0009-2614 |
| Volume | 325Issue:41035Pages:545-551 |
| Subject Area | Physics |
| Indexed By | SCI |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.itp.ac.cn/handle/311006/12921 |
| Collection | SCI期刊论文 |
| Corresponding Author | Iwamoto, M , Tokyo Inst Technol, Dept Phys Elect, Meguro Ku, 2-12-1 Ookayama, Tokyo 1528552, Japan. |
| Recommended Citation GB/T 7714 | Iwamoto, M,Wu, CX,Zhong-Can, OY,et al. Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression[J]. CHEMICAL PHYSICS LETTERS,2000,325(41035):545-551. |
| APA | Iwamoto, M,Wu, CX,Zhong-Can, OY,&Iwamoto, M , Tokyo Inst Technol, Dept Phys Elect, Meguro Ku, 2-12-1 Ookayama, Tokyo 1528552, Japan..(2000).Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression.CHEMICAL PHYSICS LETTERS,325(41035),545-551. |
| MLA | Iwamoto, M,et al."Second-order susceptibility tensor of a monolayer at the liquid-air interface: SHG spectroscopy by compression".CHEMICAL PHYSICS LETTERS 325.41035(2000):545-551. |
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| Second-order suscept（116KB） | 开放获取 | License | Application Full Text | |||
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