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题名: Reversible transient nucleation in ionic solutions as the precursor of ion crystallization
作者: Ren, G ;  Wang, YT
刊名: EPL
出版日期: 2014
卷号: 107, 期号:3, 页码:30005
关键词: HOMOGENEOUS NUCLEATION ;  ELECTROLYTE-SOLUTIONS ;  ACTIVITY-COEFFICIENTS ;  AQUEOUS-SOLUTIONS ;  DYNAMICS ;  PHASE ;  SIMULATION ;  AGGREGATION ;  CRITICALITY ;  CRYSTALS
学科分类: Physics
DOI: 10.1209/0295-5075/107/30005
通讯作者: Ren, G (reprint author), Chinese Acad Sci, Inst Theoret Phys, State Key Lab Theoret Phys, 55 East Zhongguancun Rd,POB 2735, Beijing 100190, Peoples R China.
部门归属: [Ren, Gan] Chinese Acad Sci, Inst Theoret Phys, State Key Lab Theoret Phys, Beijing 100190, Peoples R China ;  Chinese Acad Sci, Kavli Inst Theoret Phys China, Beijing 100190, Peoples R China
英文摘要: Molecular dynamics simulations for aqueous sodium chloride solutions were carried out at various concentrations. Supplementary to the Debye-Huckel theory, reversible transient nucleation of ions was observed even in dilute solutions. The average size of formed ion clusters and the lifetime of ion pairs increases with concentration until the saturation point, when ion clusters become stable and individual ions adjust their positions to form ordered lattice structures, leading to irreversible ion crystallization, which is beyond the description of the classical nucleation theory. Copyright (C) EPLA, 2014
资助者: National Basic Research Program of China (973 program) [2013CB932804]; National Natural Science Foundation of China [91227115, 11121403]; Hundred Talent Program of the Chinese Academy of Sciences (CAS)
收录类别: SCI
原文出处: 查看原文
语种: 英语
WOS记录号: WOS:000340780100005
Citation statistics: 
内容类型: 期刊论文
URI标识: http://ir.itp.ac.cn/handle/311006/15692
Appears in Collections:理论物理所2014年知识产出 _期刊论文

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Recommended Citation:
Ren, G,Wang, YT. Reversible transient nucleation in ionic solutions as the precursor of ion crystallization[J]. EPL,2014,107(3):30005.
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