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Ren, G; Wang, YT; Ren, G (reprint author), Chinese Acad Sci, Inst Theoret Phys, State Key Lab Theoret Phys, 55 East Zhongguancun Rd,POB 2735, Beijing 100190, Peoples R China.
Reversible transient nucleation in ionic solutions as the precursor of ion crystallization
发表期刊EPL
语种英语
关键词Homogeneous Nucleation Electrolyte-solutions Activity-coefficients Aqueous-solutions Dynamics Phase Simulation Aggregation Criticality Crystals
摘要Molecular dynamics simulations for aqueous sodium chloride solutions were carried out at various concentrations. Supplementary to the Debye-Huckel theory, reversible transient nucleation of ions was observed even in dilute solutions. The average size of formed ion clusters and the lifetime of ion pairs increases with concentration until the saturation point, when ion clusters become stable and individual ions adjust their positions to form ordered lattice structures, leading to irreversible ion crystallization, which is beyond the description of the classical nucleation theory. Copyright (C) EPLA, 2014
2014
ISSN0295-5075
卷号107期号:3页码:30005
学科领域Physics
DOI10.1209/0295-5075/107/30005
收录类别SCI
项目资助者National Basic Research Program of China (973 program) [2013CB932804]; National Natural Science Foundation of China [91227115, 11121403]; Hundred Talent Program of the Chinese Academy of Sciences (CAS) ; National Basic Research Program of China (973 program) [2013CB932804]; National Natural Science Foundation of China [91227115, 11121403]; Hundred Talent Program of the Chinese Academy of Sciences (CAS) ; National Basic Research Program of China (973 program) [2013CB932804]; National Natural Science Foundation of China [91227115, 11121403]; Hundred Talent Program of the Chinese Academy of Sciences (CAS) ; National Basic Research Program of China (973 program) [2013CB932804]; National Natural Science Foundation of China [91227115, 11121403]; Hundred Talent Program of the Chinese Academy of Sciences (CAS)
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文献类型期刊论文
条目标识符http://ir.itp.ac.cn/handle/311006/15692
专题理论物理所科研产出_SCI论文
通讯作者Ren, G (reprint author), Chinese Acad Sci, Inst Theoret Phys, State Key Lab Theoret Phys, 55 East Zhongguancun Rd,POB 2735, Beijing 100190, Peoples R China.
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GB/T 7714
Ren, G,Wang, YT,Ren, G . Reversible transient nucleation in ionic solutions as the precursor of ion crystallization[J]. EPL,2014,107(3):30005.
APA Ren, G,Wang, YT,&Ren, G .(2014).Reversible transient nucleation in ionic solutions as the precursor of ion crystallization.EPL,107(3),30005.
MLA Ren, G,et al."Reversible transient nucleation in ionic solutions as the precursor of ion crystallization".EPL 107.3(2014):30005.
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