Knowledge Management System of Institute of Theoretical Physics, CAS
Su, Cheng; Zeng, Xu-Tao; Li, Yi1,2; Ma, Nvsen; Lin, Zhengwang; Zhang, Chuandi; Wang, Chin-Wei; Chen, Ziyu; Lu, Xingye1,2; Li, Wei4![]() | |
Zigzag magnetic order in a novel tellurate compound Na4-delta NiTeO6 with S=1 chains | |
Source Publication | SCIENCE CHINA-PHYSICS MECHANICS & ASTRONOMY
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Language | 英语 |
Keyword | SPIN-PEIERLS TRANSITION GROUND-STATE EXCITATIONS CRYSTAL ABSENCE PHASE NI |
Abstract | Na4-delta NiTeO6 is a rare example in the transition-metal tellurate family of realizing an S = 1 spin-chain structure. By performing neutron powder diffraction measurements, the ground-state magnetic structure of Na4-delta NiTeO6 is determined. These measurements reveal that below T-N similar to 6.8(2) K, the Ni2+ moments form a screwed ferromagnetic (FM) spin-chain structure running along the crystallographic a axis but these FM spin chains are coupled antiferromagnetically along the b and c directions, giving rise to a magnetic propagation vector of k = (0, 1/2, 1/2). This zigzag magnetic order is well supported by first-principles calculations. The moment size of Ni2+ spins is determined to be 2.1(1)mu(B) at 3 K, suggesting a significant quenching of the orbital moment due to the crystalline electric field (CEF) effect. The previously reported metamagnetic transition near H-C similar to 0.1 T can be understood as a field-induced spin-flip transition. The relatively easy tunability of the dimensionality of its magnetism by external parameters makes Na4-delta NiTeO6 a promising candidate for further exploring various types of novel spin-chain physics. |
2022 | |
ISSN | 1674-7348 |
Volume | 65Issue:9Pages:297511 |
Cooperation Status | 国际 |
Subject Area | Physics |
MOST Discipline Catalogue | Physics, Multidisciplinary |
DOI | 10.1007/s11433-022-1947-1 |
Indexed By | SCIE |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.itp.ac.cn/handle/311006/27907 |
Collection | SCI期刊论文 |
Affiliation | 1.Beihang Univ, Sch Phys, Beijing 100191, Peoples R China 2.Beijing Normal Univ, Ctr Adv Quantum Studies, Beijing 100875, Peoples R China 3.Beijing Normal Univ, Dept Phys, Beijing 100875, Peoples R China 4.Australian Nucl Sci & Technol Org, Lucas Heights, NSW 2234, Australia 5.Chinese Acad Sci, Inst Theoret Phys, CAS Key Lab Theoret Phys, Beijing 100190, Peoples R China |
Recommended Citation GB/T 7714 | Su, Cheng,Zeng, Xu-Tao,Li, Yi,et al. Zigzag magnetic order in a novel tellurate compound Na4-delta NiTeO6 with S=1 chains[J]. SCIENCE CHINA-PHYSICS MECHANICS & ASTRONOMY,2022,65(9):297511. |
APA | Su, Cheng.,Zeng, Xu-Tao.,Li, Yi.,Ma, Nvsen.,Lin, Zhengwang.,...&Jin, Wentao.(2022).Zigzag magnetic order in a novel tellurate compound Na4-delta NiTeO6 with S=1 chains.SCIENCE CHINA-PHYSICS MECHANICS & ASTRONOMY,65(9),297511. |
MLA | Su, Cheng,et al."Zigzag magnetic order in a novel tellurate compound Na4-delta NiTeO6 with S=1 chains".SCIENCE CHINA-PHYSICS MECHANICS & ASTRONOMY 65.9(2022):297511. |
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Zigzag magnetic orde(1979KB) | 期刊论文 | 出版稿 | 开放获取 | CC BY-NC-SA | Application Full Text |
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