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Su, Cheng; Zeng, Xu-Tao; Li, Yi1,2; Ma, Nvsen; Lin, Zhengwang; Zhang, Chuandi; Wang, Chin-Wei; Chen, Ziyu; Lu, Xingye1,2; Li, Wei4; Sheng, Xian-Lei; Jin, Wentao
Zigzag magnetic order in a novel tellurate compound Na4-delta NiTeO6 with S=1 chains
Source PublicationSCIENCE CHINA-PHYSICS MECHANICS & ASTRONOMY
Language英语
KeywordSPIN-PEIERLS TRANSITION GROUND-STATE EXCITATIONS CRYSTAL ABSENCE PHASE NI
AbstractNa4-delta NiTeO6 is a rare example in the transition-metal tellurate family of realizing an S = 1 spin-chain structure. By performing neutron powder diffraction measurements, the ground-state magnetic structure of Na4-delta NiTeO6 is determined. These measurements reveal that below T-N similar to 6.8(2) K, the Ni2+ moments form a screwed ferromagnetic (FM) spin-chain structure running along the crystallographic a axis but these FM spin chains are coupled antiferromagnetically along the b and c directions, giving rise to a magnetic propagation vector of k = (0, 1/2, 1/2). This zigzag magnetic order is well supported by first-principles calculations. The moment size of Ni2+ spins is determined to be 2.1(1)mu(B) at 3 K, suggesting a significant quenching of the orbital moment due to the crystalline electric field (CEF) effect. The previously reported metamagnetic transition near H-C similar to 0.1 T can be understood as a field-induced spin-flip transition. The relatively easy tunability of the dimensionality of its magnetism by external parameters makes Na4-delta NiTeO6 a promising candidate for further exploring various types of novel spin-chain physics.
2022
ISSN1674-7348
Volume65Issue:9Pages:297511
Cooperation Status国际
Subject AreaPhysics
MOST Discipline CataloguePhysics, Multidisciplinary
DOI10.1007/s11433-022-1947-1
Indexed BySCIE
Citation statistics
Document Type期刊论文
Identifierhttp://ir.itp.ac.cn/handle/311006/27907
CollectionSCI期刊论文
Affiliation1.Beihang Univ, Sch Phys, Beijing 100191, Peoples R China
2.Beijing Normal Univ, Ctr Adv Quantum Studies, Beijing 100875, Peoples R China
3.Beijing Normal Univ, Dept Phys, Beijing 100875, Peoples R China
4.Australian Nucl Sci & Technol Org, Lucas Heights, NSW 2234, Australia
5.Chinese Acad Sci, Inst Theoret Phys, CAS Key Lab Theoret Phys, Beijing 100190, Peoples R China
Recommended Citation
GB/T 7714
Su, Cheng,Zeng, Xu-Tao,Li, Yi,et al. Zigzag magnetic order in a novel tellurate compound Na4-delta NiTeO6 with S=1 chains[J]. SCIENCE CHINA-PHYSICS MECHANICS & ASTRONOMY,2022,65(9):297511.
APA Su, Cheng.,Zeng, Xu-Tao.,Li, Yi.,Ma, Nvsen.,Lin, Zhengwang.,...&Jin, Wentao.(2022).Zigzag magnetic order in a novel tellurate compound Na4-delta NiTeO6 with S=1 chains.SCIENCE CHINA-PHYSICS MECHANICS & ASTRONOMY,65(9),297511.
MLA Su, Cheng,et al."Zigzag magnetic order in a novel tellurate compound Na4-delta NiTeO6 with S=1 chains".SCIENCE CHINA-PHYSICS MECHANICS & ASTRONOMY 65.9(2022):297511.
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